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<p class="MsoNormal" align="center" style="text-align:center"><b>Flexible and Stretchable Lithium-Ion Batteries Based on Solid Polymer
Nanocomposite Electrolyte<o:p></o:p></b></p>
<p class="MsoNormal" align="center" style="text-align:center">Mejdi Kammoun<o:p></o:p></p>
<p class="MsoNormal" align="center" style="text-align:center"><b>Defense Date:</b> Monday, December 5th
2016 <o:p></o:p></p>
<p class="MsoNormal" align="center" style="text-align:center"><b>Time:</b> 9:00AM <o:p></o:p></p>
<p class="MsoNormal" align="center" style="text-align:center"><b>Location:</b> Large Conference Room ME Department<o:p></o:p></p>
<p class="MsoNormal" align="center" style="text-align:center"><b>Committee members:</b> Dr. Haleh Ardebili, Dr. Yashashree Kulkarni, Dr.
Jae-Hyun Ryou, Dr. Dong Liu, Dr. Yan Yao<o:p></o:p></p>
<p class="MsoNormal"><b>Abstract<o:p></o:p></b></p>
<p class="MsoNormal">The prevalence of flexible electronics including the
ubiquitous touch-screens, roll-up displays, implantable medical devices and
wearable sensors has motivated the development of high performance flexible
energy storage devices. High energy density lithium-ion batteries (LIBs) are
the leading candidates to convert into flexible and stretchable batteries to
integrate with the flexible and stretchable applications. The ultimate
challenge is to obtain mechanical flexibility while conserving the high
electrochemical performance of conventional LIBs including high capacity and
cycling stability.<o:p></o:p></p>
<p class="MsoNormal">In this study, two types of polymer nanocomposite
electrolytes are investigated for battery and fuel cell applications. The first
polymer studied is based on Nafion, and a key problem in PEMFCs is the
dehydration of Nafion and the subsequent low performance especially at higher
temperatures. We introduced a bio-friendly coconut shell activated carbon (AC)
nanoparticles into the Nafion membranes. We showed that a small amount (i.e.
0.7%) of AC nanofillers could dramatically enhance proton conductivity without
significantly compromising the mechanical properties.<o:p></o:p></p>
<p class="MsoNormal">The second type of polymer for lithium-ion battery
application is based on the polyethylene oxide (PEO)|Li salt system. It offers
enhanced safety, stability and thin-film manufacturability compared to the
traditional organic liquid electrolytes. The electrochemical properties of the
pure polymer are improved by adding 1% graphene oxide (GO) nanosheets. We
developed a high performance flexible Li ion battery based on the solid polymer
nanocomposite electrolyte. The flexible
battery exhibits a capacity higher than 0.1 mAh/cm2 at 1 mA current and
excellent cycling stability over 100 charge/discharge cycles. <o:p></o:p></p>
<p class="MsoNormal">PEO/GO electrolyte was also incorporated in a novel design
of spiral stretchable battery capable of large out-of-plane deformation. The
spiral Li-ion battery displays robust mechanical stretchability and an energy
density of 4.862 mWh/cm3 at 650% out-of-plane deformation and provides an
average capacity above 0.1 mAh/cm2 in different stretching configurations. <o:p></o:p></p>
<p class="MsoNormal">We also investigated the temperature effects on solid polymer
electrolyte based batteries. A 1-D LIB model that predicts the discharge
behavior of coin cell batteries at different temperatures was developed. The
modeling simulations based on electrochemical-thermal coupling show good
agreement with experimental results and provide fundamental insights on the
battery operation at different conditions.<o:p></o:p></p>
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